BSTRACTThis paper presents an overview on the peculiar microstructural design

called ‘harmonic structure’ (HS)

for improved mechanical performance of structural materials. A well designed powder metallurgy processing approach has been developed to create a unique three-dimensionally gradient HS with controlled bimodal grain size distribution in metals and alloys. The bulk materials with HS exhibited considerably higher strength and improved toughness as compared to coarse-grained structures. The unique HS design promotes uniformity of deformation by avoiding strain localization during plastic deformation. A possible mechanism of deformation behavior of HS has also been proposed based on the available experimental results.