Ge Li, Ping Wang, Chenyu Li, et al. Cobalt–nickel layered double hydroxide on hollow Co3S4/CuS derived from ZIF-67 for efficient overall water splitting[J]. Materials Research Letters, 2022, 10(11): 744-753.
DOI:
Ge Li, Ping Wang, Chenyu Li, et al. Cobalt–nickel layered double hydroxide on hollow Co3S4/CuS derived from ZIF-67 for efficient overall water splitting[J]. Materials Research Letters, 2022, 10(11): 744-753.DOI: 10.1080/21663831.2022.2095235.
Cobalt–nickel layered double hydroxide on hollow Co3S4/CuS derived from ZIF-67 for efficient overall water splitting
Electrochemical water splitting is one of the most efficient strategies to generate clean energy H
2
. Herein
a novel hollow Co
3
S
4
/CuS@CoNi-LDH nanocomposite was designed. This hollow Co
3
S
4
/CuS@CoNi-LDH achieved OER overpotential of 220 mV
HER overpotential of 136 mV
respectively
at the current density of 10 mA cm
−2
. Notably
the hollow Co
3
S
4
/CuS@CoNi-LDH serving as both anode and cathode is assembled into a two-electrode water splitting device
and the potential of no more than 1.74 V is required to achieve the overall water splitting efficiency of 10 mA cm
−2
. This work provides a promising bifunctional catalyst for overall electrochemical water splitting.
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references
Al-Qirby LM, Radiman S, Siong CW, et al. Sonochemical synthesis and characterization of Co3O4 nanocrystals in the presence of the ionic liquid [EMIM][BF4]. Ultrason Sonochem. 2017;38:640–651. (Open in a new window)PubMed (Open in a new window)Web of Science ®(Open in a new window)Google Scholar
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